It's not typically connected to the frame itself directly, but rather to a specifically designed grounding point that's attached to the frame. Look for a substantial bolt, often painted black, that's easily accessible and shows signs of being used as a ground.
If you're unsure, consult a wiring diagram specific to your 1991 Jeep Wrangler. A repair manual (Haynes or Chilton are good options) would be very helpful in locating this ground point accurately. You can also often find diagrams online, but verify the accuracy by cross-referencing several sources.